One‐Pot Synthesis of Melt‐Processable Supramolecular Soft Actuators

نویسندگان

چکیده

Abstract The application of reprocessable and reprogrammable soft actuators is limited by the synthetic strategies, 3D‐shaping capabilities, small deformations. In this work, melt‐processable supramolecular based on segmented copolymers containing thiourethane liquid crystal segments have been prepared via sequential thiol addition reactions in a one‐pot approach using commercially available building blocks. demonstrated immediate, reversible response weightlifting capabilities with large deformations up to 32 %. Through exploiting cross‐links, material could be recycled reprogrammed into 3D welded an actuator assembly different deformation modes. Our work offers synthesis straightforward prepare that can reprocessed arbitrary shapes.

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ژورنال

عنوان ژورنال: Angewandte Chemie

سال: 2021

ISSN: ['1521-3773', '1433-7851', '0570-0833']

DOI: https://doi.org/10.1002/ange.202115166